Chemical Science

List of Papers (Total 4,436)

Selective coordination of three transition metal ions within a coiled-coil peptide scaffold.

Designing peptides that fold and assemble in response to metal ions tests our understanding of how peptide folding and metal binding influence one another. Here, histidine residues are introduced into the hydrophobic core of a coiled-coil trimer, generating ...

Dynamic colloidal nanoparticle assembly triggered by aptamer-receptor interactions on live cell membranes.

Cells use dynamic systems such as enzyme cascades and signaling networks to control cellular functions. Synthetic dynamic systems that can be target-responsive have great potential to be applied for biomedical applications but the operation of such dynamic ...

Visible-light-mediated deuteration of silanes with deuterium oxide.

Isotopically labeled compounds are highly desirable as they can serve as both mechanistic probes in chemistry and diagnostic tools in medicinal research. Herein, we report an unprecedented visible-light-mediated metal-free deuteration of silanes using ...

Organobase triggered controlled supramolecular ring opening polymerization and 2D assembly.

Spontaneously aggregation of a carboxylic acid appended NDI can be retarted by intra-molecular H-bonding. With catalytic DMAP or DBU, the meta-stable monomer exhibits living supramolecular polymerization and generates ultra-thin 2D sheet.A carboxylic ...

Towards high energy density lithium battery anodes: silicon and lithium.

Silicon and lithium metal are considered as promising alternatives to state-of-the-art graphite anodes for higher energy density lithium batteries because of their high theoretical capacity. However, significant challenges such as short cycle life and ...

Introduction of the α-ketoamide structure: en route to develop hydrogen peroxide responsive prodrugs.

New light on H[2] O[2] -activated prodrugs: the first α-ketoamide based prodrug opens up new alternatives for designing non-boron based H[2] O[2] -responsive promoieties.Leveraging the elevated levels of hydrogen peroxide (H[2] O[2] ) in cancer, ...

Expanding the mass range for UVPD-based native top-down mass spectrometry.

Native top-down mass spectrometry is emerging as a methodology that can be used to structurally investigate protein assemblies. To extend the possibilities of native top-down mass spectrometry to larger and more heterogeneous biomolecular assemblies, ...

Molecular recognition of planar and non-planar aromatic hydrocarbons through multipoint Ag-π bonding in a dinuclear metallo-macrocycle.

Exploration of a novel structural motif of host–guest interactions is one of the most fundamental topics to develop macrocycle-based host–guest/supramolecular systems. Herein, we present an unprecedented mode of inclusion of aromatic hydrocarbons ...

Tetragonal phosphorus(v) cations as tunable and robust catalytic Lewis acids.

The synthesis and catalytic reactivity of a class of water-tolerant cationic phosphorus-based Lewis acids is reported. Corrole-based phosphorus() cations of the type [ArP(cor)][B(C[6] F[5] )[4] ] (Ar = C[6] H[5] , 3,5-(CF[3] )[2] C[6] H[3] ; cor = 5,10,15-(C[6] ...

Catalytic Au(i)/Au(iii) arylation with the hemilabile MeDalphos ligand: unusual selectivity for electron-rich iodoarenes and efficient application to indoles.

The ability of the hemilabile (P,N) MeDalphos ligand to trigger oxidative addition of iodoarenes to gold has been thoroughly studied. Competition experiments and Hammett correlations substantiate a clear preference of gold for electron-enriched substrates ...

Antimicrobial silver targets glyceraldehyde-3-phosphate dehydrogenase in glycolysis of E. coli.

We report for the first time that antimicrobial Ag[+] targets the glycolytic pathway through inhibiting the key enzyme of GAPDH.Silver has long been used as an antibacterial agent, yet its molecular targets remain largely unknown. Using a custom-designed ...

Towards large scale hybrid QM/MM dynamics of complex systems with advanced point dipole polarizable embeddings.

In this work, we present a general route to hybrid Quantum Mechanics/Molecular Mechanics (QM/MM) Molecular Dynamics for complex systems using a polarizable embedding. We extend the capabilities of our hybrid framework, combining the Gaussian and Tinker/Tinker-HP ...

Conformational diversity induces nanosecond-timescale chemical disorder in the HIV-1 protease reaction pathway.

One enzyme, one substrate, but two different reaction mechanisms: HIV-1 protease follows different reaction mechanisms depending on its instantaneous conformation.The role of conformational diversity in enzyme catalysis has been a matter of analysis ...

Enhanced three-photon activity triggered by the AIE behaviour of a novel terpyridine-based Zn(ii) complex bearing a thiophene bridge.

Multiphoton bioimaging benefits from good penetration of tissue, low phototoxicity and high resolution. Hence, development of efficient multiphoton imaging agents is highly desirable but remains challenging. Herein, a novel terpyridine-based Zn() complex ...

Covalency and magnetic anisotropy in lanthanide single molecule magnets: the DyDOTA archetype.

Lanthanide ions when complexed by polyamino-polycarboxylate chelators form a class of compounds of paramount importance in several research and technological areas, particularly in the fields of magnetic resonance and molecular magnetism. Indeed, the ...

Palladium-catalyzed enantioselective alkenylation of alkenylbenzene derivatives.

A regioselective and enantioselective palladium-catalyzed relay Heck alkenylation of alkenylbenzene derivatives to construct remote stereocenters is disclosed. Various β-substituted styrenes were readily obtained in moderate yields with good to ...

Substituent-controlled, mild oxidative fluorination of iodoarenes: synthesis and structural study of aryl I(iii)- and I(v)-fluorides.

We report a mild approach to the synthesis of difluoro(aryl)-λ[3] -iodanes (aryl-IF[2] compounds) and tetrafluoro(aryl)-λ[5] -iodanes (aryl-IF[4] compounds) using trichloroisocyanuric acid (TCICA) and potassium fluoride (KF). Under these ...

The S∴π hemibond and its competition with the S∴S hemibond in the simplest model system: infrared spectroscopy of the [benzene-(H2S) n ]+ (n = 1-4) radical cation clusters.

The S∴π hemibond (two-center three-electron, 2c-3e, bond) is an attractive interaction between a sulfur atom and π electrons. The S∴π hemibond is of essential importance in understanding chemistry of sulfur radical ...

Active template rotaxane synthesis through the Ni-catalyzed cross-coupling of alkylzinc reagents with redox-active esters.

The synthesis of unsymmetrical axle [2]rotaxanes through a recently developed Ni-catalyzed C(sp[3] )–C(sp[3] ) cross-coupling of redox-active esters (formed directly from carboxylic acids) and organozinc reagents (derived from alkyl bromides) ...

Photolytic, radical-mediated hydrophosphination: a convenient post-polymerisation modification route to P-di(organosubstituted) polyphosphinoboranes [RR'PBH2] n.

New, air-stable inorganic soft materials are accessible under mild conditions via TEMPO-mediated radical hydrophosphination of alkenes using polyphosphinoboranes.Polymers with a phosphorus-boron main chain have attracted interest as novel inorganic materials ...

A Janus-inspired amphichromatic system that kills two birds with one stone for operating a "DNA Janus Logic Pair" (DJLP) library.

Although DNA computing has exhibited a magical power across diverse areas, current DNA logic gates with different functions are always separately operated and can only produce hard-to-visualize output. The fussy/obligatory gates

Strategies based on metal-based nanoparticles for hypoxic-tumor radiotherapy.

Radiotherapy (RT) is one of the most effective and frequent clinical cancer treatments. Nevertheless, RT can cause damage to normal tissues around tumors under high-dose ionizing radiation. Inspired by versatile metal-based nanomaterials, great efforts ...

Glycerol transport through the aquaglyceroporin GlpF: bridging dynamics and kinetics with atomic simulation.

The aquaglyceroporin GlpF is a member of the aquaporin family. It selectively conducts small molecules, such as glycerol, across the cell membrane under a concentration gradient of the substrate. Atomistic molecular dynamics (MD) simulation would provide ...

Pushing the analytical limits: new insights into complex mixtures using mass spectra segments of constant ultrahigh resolving power.

A new strategy has been developed for characterization of the most challenging complex mixtures to date, using a combination of custom-designed experiments and a new data pre-processing algorithm. In contrast to traditional methods, the approach enables ...

Aza-proline effectively mimics l-proline stereochemistry in triple helical collagen.

Chenoweth and co-workers provide an atomic resolution crystal structure and computational analysis illustrating that aza-proline mimics -proline stereochemistry in collagen.The prevalence of -amino acids in biomolecules has been shown to have teleological ...